Fe(Te1-xSex), optimal doping for superconductivity (x~0.4-0.5)

(For FeSe, i.e., x = 1, see this page 🔗.)

Structure

Crystal Image

Crystal Structure

The real samples usually have excess Fe at the interstitial sites of the Te/Se layer, forming Fe1+y(Te1-xSex) composition. Such excess affects the magnetic and electronic transport properties.

XRD

Single-crystal and power spectrum for Fe1.03(Te0.6Se0.4)

XRD

Single-crystal spectrum (00L reflections) for Fe1.03(Te1-xSex)

Structural property summary

  • Single crystal form: silver color, metallic luster, square/rectangle facets
  • Structure type: Layered, P4/nmm
  • Air sensitivity: stable
  • Exfoliation: very easy

Transport Properties

Resistivity- Temperature dependence

  • The transition temperature and metallicity in the normal state are greatly affected by sample quality, amount of excess Fe, and Se:Te ratio.
  • Excess Fe induces (pi, 0) magnetic fluctuations, suppresses transition temperature, and suppresses metallicity in the normal state.
  • For minimized excess Fe (< 2%), the properties (transport, magnetization, and specific heat) are similar for samples with Se:Te ratio in the range of 0.35:0.65 – 0.5:0.5

Magnetic Properties

Magnetization- Temperature dependence

Meissner effect

Specific Heat

Specific Heat (C vs T)

The transition temperature and specific jump are greatly affected by sample quality and Se:Te ratio

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